I've watched every available adaptation,
and it's a tie between this and the 1973 BBC miniseries for my favorite. It's not just because it includes most of the book, but because of that, it does tell the story better and really brings the dialogue in the book to life. I think the acting is better, especially both Rochesters. Timothy Dalton brings a lot of passion to the character that I can picture in the book and Jayston does a great job, too. It's unfortunate about Jayston's eyeliner, my only complaint.
These are the other ones I watched, 1934, 1943, 1970, 1996, 1997, 2006, 2011.