Depending on his ability to acquire a food source, what COULDN'T he eat? Once you're down to that size, it hardly takes much of a normal-sized food source to fill you up!
But as he shrank to molecular size, there wouldn't be food for him, because food (and everything) is made up of a combination of different molecules/atoms/whathaveyou. (I AM NOT A SCIENTIST!)
But, the point is, he would eventually reach a tiny state where there was nothing left to eat because the particles that make up food would be individualized, and not actual foods any more. So there would be no "food" to eat.
For instance, if water is hydrogen and oxygen, he would eventually be facing those two elements individually....not the combination of them that equal "water"....right?
At that point, he would starve/die from thirst.
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